I wanted to give a brief update on this.
The Center (round 1), and the 2 sequentially numbered CX-17's were recapped (round 3 and 4, one of which was the problem child). The TimeFrames are being ran as is, mainly because they still sound great and the replacement poly cap that was ordered was prohibitively huge. I can now see why others go for another electrolytic in this application, however I plan to address this down the line, as these speakers deserve the refinishing they are in need of. I am not sure if the problem child is completely fixed because of the recap, because I haven't had a chance to do any extensive testing. They were pretty much recapped, verified that both drivers were still working, and plopped in rear speaker mounts.
For setup, everything is being driven by a Sony STR-DE597 receiver (90WPCx6, Surround center unused), and being backed by a Sony SA-WM40 powered sub (12", 120watt). The cutoff on the receiver was set to 80hz based on internet research. For music, the system is incredible, but we are running in to one issue, bass, or namely, too much of it in all the wrong frequencies. I likely need to readdress the cutoff frequency and subwoofer approach. I wasn't able to get to deep in to this because my mother returned home soon after initial setup, with a migraine, and NO tolerance for the noises that were being made in her living room.
So far, it sounds like some great noises are being made, it's all a matter of tuning from here.