Well -- in the absence of any other data on these speakers... what I would probably do is borrow (or buy) a decent "LCR" meter to measure the
actual capacitance of each XO capacitor.
Now -- each of the
two capacitors in the "good" speaker crossover
only has two leads (wires) sticking out of it, yes? I ask because (especially in the 1960s) it wasn't uncommon to find dual capacitors in one package used for speaker crossovers (KLH comes to mind). A dual capacitor would probably have
three leads, and maybe even
four.
Take plenty of photographs to be
100% sure that you know how the original crossovers were wired, then snip out
one capacitor and measure its
actual capacitance with the meter. Use the leads provided with the meter
or use test leads as short as possible. Chances are the "actual" capacitance of each capacitor is still within a factor of 2 or so of the
intended value.
Do that for each of the two capacitors and then order a selection of capacitors "around" the actual values. E.g., suppose you measure one to be 5 uF. Order, say, a 2 uF, a 5 uF and a 10 uF.
IF the crossovers are first order (and, given what "we" know right now, that's
not a given) the crossover frequency, fc, is given by this equation:
fc = 1 / (2 * pi * R * C)
where pi = 3.14159265... (good old π)
R = the load (speaker driver) impedance
C = the capacitor value (in Farads -- one Farad = 1,000,000 uF)
This is the equation used by the crossover calculators.
From this equation, and for a 8 ohm speaker driver (R = 8), we can see a 1 uF capacitor corresponds to fc = 20,000 Hz, for example.
Similarly:
C = 2 uF corresponds to fc = 10,000 Hz
C = 5 uF corresponds to fc = 4,000 Hz
C = 10 uF corresponds to fc = 2,000 Hz
C = 20 uF corresponds to fc = 1,000 Hz
etc.
My suggestion: If you go this route, buy a bunch of cheap nonpolarized electrolytics for your experiments.
If you find values you like,
and if you really like the loudspeakers, then go back and invest in better quality XO capacitors at the values you chose.
I've gotta say I am baffled by these speakers

You might want to ask about them at a site such as DIY HiFi...(?)
To put these crossover numbers into perspective, here's how the notes on a piano keyboard correlate to
fundamental frequencies.