BuzzK: I'm curious as to what you would hope to obtain by doing the crossover upgrade. Are your L100's in good shape as they are?
I've had two pair of 4311's, two pair of 4312's, and one pair of L100's. I've always felt that, to my ears at least, the midrange from all of these speakers was pretty good but one had to be careful with the tweeter, especially on the 4312's. As far as bass is concerned, none of them had quite enough for me.
In a last-ditch effort to get the kind of sound I was looking for, I purchased a Polk PSW-505 subwoofer and added that to one of my systems using a Yamaha receiver and a pair of 4312's. I kept all of the level controls on the speakers right at their midpoint and I did the same with the subwoofer's crossover and volume controls.
The results, at least to me, were pretty damn good! I'm very happy with this particular system and I find that I use it almost exclusively for vinyl. The midrange is still top-notch, but now I have some "warmth" to the music, especially the vocals. In combination with keeping the tweeter levels down somewhat, I find the sound to be just right for most of my vinyl. Occasionally I'll have to make a minor adjustment here or there on certain records.
The reason I bring all of this up is because, for $199 (amazon.com), I improved my system to where I wished it to be with a minimum of fuss. I've always been skeptical of the crossover upgrades. Oh, I'm sure they work, and probably work well in some cases, but for "older ears," I'm not sure if one could tell much difference from the original sound of the speakers.
Just a thought.