Haven't pulled the 2270 down for this yet, but you are right, that's next on the list.
And in fact, you hit the nail on the head here - I think the brightness of Klipsch can be offset and in fact utilized with an older Marantz receiver. There's no doubt those silver-faced Marantz have their own warm sound. I'm really excited to bring it down off the shelf and try it out.
I have no problem using the tone controls when hitting my final config, but so far, it's been the "direct" mode that I usually use in this system.
Currently, as you know, I'm driving these with a Marantz SR-4023 (fed with a decent SACD). The local audio shop of course is biased, but they have had a 4023 near the front of their display, hooked to a variety of speakers for over a year now - it sounds good enough and price low enough for people to either buy or move deeper into the store, they say.
Next up, maybe some Devo with their tight drum. Already got all the floyd SACD's stacked and ready for the right listening time.
If I had a friend with a 4 way+ setup like you, I'd spend hundreds of hours there too! I bet it sounds great, like you say, it's set up properly too. Nice.
I'll also say - downstairs, in my basement is the man-cave. Threw in some KP-201's as mains with a $300 Klipsch sub, and hooked to a $300 Onkyo cheapie HT unit. I am continually impressed with how good it sounds for stereo music. Obviously part of it is the room, but I can't believe how good that damn Onkyo sounds. None of my other systems sound as good. Damn room. Pissed me off. LOL.
Have you played the KLF with your Marantz 2270? It has 3 tone knobs one for each separate driver types in the cabinet. Adjust each one until you like the "Balanced" sound. Reduce the gain on the mids and tweeter and see what it sounds like. I had a Marantz 2285B many years ago and loved it on my Heresy II.YMMV on the KLF-20. My Yamaha A-1000 Class A Integrated Amp I use on my Cornwalls for analog has tone controls that I use on about every different vintage LP I clean and play. I have spent hundreds of hours and my friends house with his 4 KLF-20/C7 SVS sub and plays his stereo music thru a Bluray player and his Yamaha AVR and it sounds Great. ( I know a terrible thing to do

) HT even better after his runs the room correction program(YAPO) and then a hand held sound meter and manual adjusts the AVR Eq. for his room and his hearing. I Can make either of my Klipsch speakers sound so Harsh and Bright with the mid and tweeter tone controls maxed out that they will bore a hole in your head in this small room. Start out with all three tone controls set flat or at 1/2 of the rotation and give it listen.
And adjust for the room and you. Enjoy those KLF-20, they are great speakers.